From: THE MAMMOTH TRUMPET (March 2001)
TERRESTRIAL EVIDENCE OF A NUCLEAR CATASTROPHE IN PALEOINDIAN TIMES
[PDF version includes tables, figures, etc.]
[updated response to post publication questions][.doc version]
by Richard B. Firestone, Lawrence
Berkeley National Laboratory,
and William Topping, Consultant,
THE PALEOINDIAN OCCUPATION of North America, theoretically the point of entry of the first people to the Americas, is traditionally assumed to have occurred within a short time span beginning at about 12,000 yr B.P. This is inconsistent with much older South American dates of around 32,000 yr B.P.1 and the similarity of the Paleoindian toolkit to Mousterian traditions that disappeared about 30,000 years ago.2 A pattern of unusually young radiocarbon dates in the Northeast has been noted by Bonnichsen and Will.3,4 Our research indicates that the entire Great Lakes region (and beyond) was subjected to particle bombardment and a catastrophic nuclear irradiation that produced secondary thermal neutrons from cosmic ray interactions. The neutrons produced unusually large quantities of 239 Pu and substantially altered the natural uranium abundance ratios ( 235 U/238 U) in artifacts and in other exposed materials including cherts, sediments, and the entire landscape. These neutrons necessarily transmuted residual nitrogen ( 14 N) in the dated charcoals to radiocarbon, thus explaining anomalous dates.
The evidence from dated materials
We investigated a cluster of especially young radiocarbon dates concentrated in the north-central area of North America. For example, at the Gainey site in Michigan a 2880 yr B.P. radio-carbon date was reported, while the thermoluminescence date for that site is 12,400 yr B.P.5 Other anomalous dates found at Leavitt in Michigan, 6 Zander and Thedford in Ontario,7 Potts in New York,8 Alton in Indiana, 9 and Grant Lake in Nunavut 10 are summarized in Table 1. The Grant Lake Paleoindian site is most remarkable because its 160 [rc] yr B.P. age is nearly contemporary, while adjacent and deeper samples give ages of 14803620 [rc] yr B.P.
Stratigraphic associations place Paleoindian occupations at depth on the pre-historic North American landscape on sediments that form the old C horizon composed of parent material, Wisconsinan deposits that predate Holocene sediment buildup.11,12,13 The young Paleoindian dates cannot be correct, particularly since there are no patterned anomalies noted in later-period prehistoric assem-blages relating to higher stratigraphic positions. In a pioneering study of the Paleoindian site at Barnes, Michigan, Wright and Roosa observed that Paleoindian artifacts were deposited before the formation of spodosols ceased in this area about 10,000 yr B.P.14 This conclusion was based on observing that cemented sediments on artifacts, found outside their original context, defines their original stratigraphic position.
The evidence from particle bombardment
Sediment profiles were taken at Paleoindian sites and at numerous widely separated control locations in Michigan. The C sediment horizon is clearly recognized by its transitional color and confirmed by elevated concentrations of potassium and other isotopes. Color and chemistry are key indicators of this very old soil 11,12,13 derived from parent materials and associated postglacial runoff.15 At Gainey, large quantities of micrometeorite-like particles appear to be concentrated near the boundary between the B and C sediment horizons. They can be separated with a magnet and are identified by the presence of chondrules and by visual evidence of sintering and partial melting. These particles, dissimilar to common magnetites, are found in association with a high frequency of "spherules." The depth profiles for potassium and particles at the Gainey site are compared in Fig. 1. Minor vertical sorting of particles is apparent, with a shallow spike of particles near the surface probably resulting from modern agricultural or industrial activity. Total gamma-ray counting of sediment profiles in the various locations invariably showed increased radioactivity at the B-C boundary consistent with enhanced potassium ( 40 K) and possibly other activities.
Microscopic examination of chert artifacts from several widely separated Paleoindian locations in North America revealed a high density of entrance wounds and particles at depths that are evidence of high-velocity particle bombardment. Chondrules were identified visually; their presence necessarily indicates heating during high-speed entry into the atmosphere. The depth of penetration into the artifacts implies that the particles entered with substantial energy.16 Field simulations with control cherts for large particles (100200 microns) suggest an entrance velocity greater than 0.4 km/s, and experiments at the National Superconducting Cyclotron Laboratory indicate that the smaller particles left tracks comparable to about 526 MeV iron ions ( 56 Fe) in Gainey artifacts. Similar features are not observed in later-period prehistoric artifacts or in bedrock chert sources. Track angles were estimated visually; track densities were measured with a stage micrometer; track depths were found by adjusting the microscope focus through the track. These data are summarized in Table 1.
Track and particle data in Table 1 suggest that the total track volume (density times depth) is highest at the Michigan, Illinois, and Indiana sites and decreases in all directions from this region, consistent with a widespread catastrophe concentrated over the Great Lakes region. The nearly vertical direction of the tracks left by particle impacts at most sites suggests they came from a distant source.
The evidence from uranium and plutonium
Natural uranium, which is ubiquitous in cherts, has a 235 U/238 U isotopic ratio of 0.72 percent, which varies by less than 0.1 percent in natural sources.17 Significant variations in the isotopic ratio do not occur because of chemical processes; however, a thermal neutron bombardment depletes 235 U and thus alters the ratio. Solar or galactic cosmic rays interacting with matter produce fast secondary neutrons that become thermalized by scattering from surrounding materials. Thermal neutrons see a target of large cross section (681 barns)A for destroying 235 U, compared with a target of only 2.68 barns for neutron capture on 238 U. Therefore, despite the low abundance of 235 U, about 1.8 times as many 235 U atoms are destroyed as 238 U atoms by thermal neutrons.
If a large cosmic-ray bombardment impacted the earth and irradiated the prehistoric landscape with thermal neutrons, the 235 U/238 U ratio would be changed; 239 Pu would be produced from neutron capture on 238 U, followed by the decay of 239 U. Neutrons colliding with nitrogen (1.83 barns) would create 14 C in exactly the same way 14 C is normally produced in the upper atmosphere, necessarily resetting the radiocarbon dates of any organic materials lying near the surface on the North American prehistoric landscapeincluding charcoals at Paleoindian sitesto younger values. 239 Pu produced during the bombardment will also be partly destroyed by thermal neutrons with 1017 barn cross section. Assuming 239 Pu doesnt mobilize, it will decay back to 235 U (half-life 24,110 yr), partially restoring the normal abundance.
Paleoindian artifacts from Gainey, Leavitt, and Butler, and two later-period artifacts from the same geographic area of Michigan were analyzed for 235 U content by gamma-ray counting at the Phoenix Memorial Laboratory, University of Michigan. They were compared with identical chert types representative of the source materials for the artifacts. Control samples were extracted from the inner core of the purest chert known to be utilized by prehistoric people. The Paleoindian artifacts contained about 78 percent as much 235 U as the controls and later-period artifacts, suggesting substantial depletion. Depletion of 235 U necessarily indicates that thermal neutrons impacted these artifacts and the surrounding prehistoric landscape.
Various artifacts, cherts, sediments, and a control sample containing about 0.2 percent uranium obtained from uraninite were sent to the McMaster University Centre for Neutron Activation Analysis to determine 235 U concentration by delayed neutron counting and 238 U concentration by activation analysis. These results are shown in Table 2. The 235 U/238 U ratios for all samples except the control deviated substantially from the expected ratio. McMaster ran additional calibration standards and has considerable expertise analyzing low-level uranium. This analysis was sensitive to a few ppb for 235 U and 0.10.3 ppm for 238 U, more than sufficient to precisely analyze the uranium-rich chert samples (0.7163.5 ppm). Most samples were depleted in 235 U, depletion increasing geographically from the southwest (Baker, Chuska chert, 17 percent) to the northeast (Upper Mercer, 77 percent), as shown in Table 2. This is consistent with cosmic rays focused towards northern latitudes by Earths magnetic field. Only a very large thermal neutron flux, greater than 10^20 n/cm 2 , could have depleted 235 U at all locations.
Samples of unaltered flakes from Taylor and sediment originally adjacent to Gainey artifacts showed 235 U enriched by 30 percent. Both samples were closely associated with the particles described above. The position of these samples appears to be related to the enrichment, which cannot be explained by thermal neutrons from the bombardment. To test this, we bathed another Taylor flake in 48-percent HF at 60°F for ten minutes to remove the outer 70 percent of the sample and the attached particles. Analysis showed the "inner" flake depleted in 235 U by 20 percent, consistent with the other depleted cherts.
Samples of Gainey sediment and Taylor flakes were analyzed for plutonium by Nuclear Technology Services, Inc., of Roswell, Georgia, which specializes in radiochemistry using standard methodology. The plutonium, with an aliquot of NIST-traceable 242 Pu added, was chemically separated on an anion exchange resin column and counted on an alpha-particle spectrometer. The 239 Pu/238 U ratios in both samples were approximately 10 ppb, vastly exceeding the expected ratio of 0.003 ppb.18 The results of this analysis are shown in Table 2.
Chert is a glass-like material highly impervious to penetration by any nuclear fallout that might also contribute 239 Pu. We analyzed a long-exposed piece of Bayport chert by gamma-ray counting at the LBNL low-background facility for the presence of cesium-137 ( 137 Cs), a key indicator of fallout (from nuclear testing), and found none. The B-C interface typically lies sufficiently deep that contamination by fallout is improbable. It is important to note that fallout cannot explain the depletion of 235 U.
Since the depletion of 235 U must have resulted from bombardment by thermal neutrons, the presence of 239 Pu from irradiation of 238 U is expected. The total thermal neutron flux required to produce the observed 239 Pu concentration can be cal-culated from the relative concentrations of 239 Pu (corrected for the decay) and 238 U, and the thermal neutroncapture cross section for 238 U. This neutron flux can then be used to estimate the amount of additional 14 C that would have been produced in charcoal by neutrons colliding with 14 N ( 14 N cross section = 1.83 barns). The corrected radiocarbon age can then be estimated by comparing the current amount of 14 C in the dated char-coals, determined from their measured radiocarbon age, with the amount of 14 C that would have been produced by the bombardment. For these calculations we assume that charcoal contains 0.05 per-cent residual nitrogen 19 and that initial 14 C concentrations were the same as to-day (one 14 C atom for 10^12 12 C atoms).
We derive a thermal neutron flux of c. 10^17 n/cm 2 at Gainey, which corresponds to an approximate date of 39,000 yr B.P. No radiocarbon date is available for the more southerly Taylor site, but for the conventional range of accepted Paleoindian dates the neutron flux would be c. 10^16 n/cm 2 , giving a date of about 40,000 yr B.P. These calculations necessarily neglect differences in the neutron flux experienced by the dated charcoal and the artifacts, the effects of residual 239 Pu from previous bombardments, and loss of 239 Pu due to leaching from chert over time.
The neutron flux calculated from the 235 U/238 U ratio is more than 1000 times that implied by the level of 239 Pu. Since 239 Pu decays to 235 U, partly restoring the natural abundance, it appears that substantial quantities of 239 Pu have migrated out of the chert. This mobility is demonstrated at the Nevada Test Site, where plutonium, produced in nuclear tests con-ducted by the U.S. between 1956 and 1992, migrated 1.3 km.20 It has also been shown that atoms produced by radioactive decay or nuclear reaction become weakly bound to the parent material and pass more readily into solution than isotopes not affected.21 Both 239 Pu and 235 U are thus expected to be mobile, complicating any analysis. This is consistent with the enrichment of 235 U in the two external samples where migrating 239 Pu or 235 U may have been trapped, thus enriching the relatively uranium-poor outer regions. Alternatively, excess 235 U may have been carried in by the particles. Radiocarbon produced in situ by irradiation should also be mobile. If 14 C is more mobile than 239 Pu, then the dates calculated above should be decreased accordingly.
Redating North American sites
The 39,000 yr B.P. date proposed for the Gainey site is consistent with the prevailing opinion among many archaeologists about when the Americas were populated. It is also commensurate with dates for South American sites and with a Mousterian toolkit tradition that many see as the Paleoindian precursor. The proposed date for the Gainey site also falls closer in line with the radiocarbon date for a Lewisville, Texas, Paleoindian site of 26,610 ± 300 yr B.P.22,23 and radio-carbon dates as early as c. 20,000 yr B.P. for Meadowcroft Rockshelter.24 Since the Lewisville and Meadowcroft sites were likely exposed at the same time to ther-mal neutrons, we estimate that their dates should be reset to c. 55,000 yr B.P. and c. 45,000 yr B.P., respectively.
It is likely that Paleoindians occupied low latitudes during the full glacial and migrated to more northerly areas as the ice front retreated. Therefore the pat-tern of dates makes sense from the archaeologists point of view. Dates for North American sites should generally be reset by up to 40,000 years, depending on latitude and overburden.
Geologists believe that before c. 15,000 yr B.P. the Wisconsinan glaciation covered the more northerly locations where Paleoindian sites have been found.25 The ice sheet would have shielded the landscape and any artifacts from an irradiation. (The Gainey thermoluminescence date of 12,400 yr B.P. is probably a result of the heat generated by the nuclear bombardment at that time, which would have reset the TL index to zero.) The modified dates for Paleoindian settlements suggest that the timetable for glacial advance sequences, strongly driven by conventional radiocarbon dates, should be revisited in light of the evidence presented here of much older occupations than previously thought."
The evidence from tree rings and marine sediments
A large nuclear bombardment should have left evidence elsewhere in the radio- carbon record. It is well known that radiocarbon dates are increasingly too young as we go back in time. The global Carbon Cycle suggests that 14 C produced by cosmic rays would be rapidly dispersed in the large carbon reservoirs in the atmosphere, land, and oceans.26 We would expect to see a sudden increase in radiocarbon in the atmosphere that would be incorporated into plants and animals soon after the irradiation; after only a few years, most of the radiocarbon would move into the ocean reservoirs. The 14 C level in the fossil record would reset to a higher value. The excess global radiocarbon would then decay with a half-life of 5730 years, which should be seen in the radiocarbon analysis of varved systems.
Fig. 2 plots 14 C from the INTCAL98 radiocarbon age calibration data of Stuiver et al. for 15,0000 yr B.P.27 and Icelandic marine sediment 14 C data measured by Voelker et al. for 50,00011,000 yr B.P.28 Excess 14 C is indicated by the difference between the reported radiocarbon dates and actual dates. Sharp increases in 14 C are apparent in the marine data at 40,00043,000, 32,00034,000 and c. 12,000 yr B.P These increases are coincident with geomagnetic excursions B that occurred at about 12,000 (Gothenburg), 32,000 (Mono Lake), and 43,000 yr B.P. (Laschamp),29 when the reduced magnetic field would have made Earth especially vulnerable to cosmic ray bombardment. The interstitial radiocarbon data following the three excursions were numerically fit, assuming exponential decay plus a constant cosmic rayproduced component. The fitted half-lives of 5750 yr (37,00034,000 yr B.P.), 6020 yr (32,00016,000 yr B.P.), and 6120 yr (12,0000 yr B.P.) are in good agreement with the expected value.
We also determined that contemporary radiocarbon contains about 7 percent residual 14 C left over from the catastrophe. The constant cosmic ray production rate was about 34 percent higher for the Icelandic sediment than the INTCAL98 samples, perhaps implying higher cosmic ray rates farther north. Disregarding fluctuations in the data from variations in ocean temperatures and currents, the results are clearly consistent with the decay of radiocarbon following the three geomagnetic excursions.
In Fig. 2, the sharp drop in 14 C activity before 41,000 yr B.P. suggests that global radiocarbon increased by about 45 percent at that time and by about 20 percent at 33,000 and 12,000 yr B.P The results are remarkably consistent with Vogels comparison of 14 C and U-Th dates of a stalagmite that indicates global radiocarbon increased about 75 percent from 30,000 to 40,000 yr B.P. and about 30 percent around 18,000 yr B.P.30
McHargue et al. found high levels of 10 Be in Gulf of California marine sediments at 32,000 and 43,000 yr B.P.C that could not be explained by magnetic reversal alone and were attributed to cosmic rays, possibly from a supernova.29 The geomagnetic excursion at 12,500 yr B.P. coincides with the thermoluminescence date from Gainey, and additional evidence for a cosmic ray bombardment at that time is found in the increases of 10 Be,31 Ca,32 and Mg 32 in Greenland ice cores around 12,500 yr B.P. Similar increases are also seen in the data for NO 3 , SO 4 , Mg + , Cl , K + , and Na + ions in Greenland ice cores.33 This occurrence can be dated precisely to 12,500 ± 500 yr B.P., an average of the remarkably consistent concentration peak centroids in the Greenland ice core data. Significant increases at that time are not found in comparable data for the Antarctic, which indicates that the cosmic ray irradiation was centered in the Northern Hemisphere. Weak evidence of an occurrence at 12,500 yr B.P. is seen in the radiocarbon record for marine sediments near Venezuela,34 confirming that the cosmic ray bombardment was most severe in northern latitudes.
Lunar cosmogenic data also show evidence of increased solar cosmic ray activity at or before 20,000 yr B.P.35,36 although these data are not sensitive to earlier irradiation.
The effect of a supernova on Earth
Sonett suggests that a single supernova would produce two or three shock waves, an initial forward shock and a pair of reverse shocks from the initial expansion and a reflected wave from the shell boundary of a more ancient supernova.39,40 Fig. 2 shows that each episode in a series produced a similar amount of atmospheric radiocarbon. The sun lies almost exactly in the center 41 of the Local Bubble, believed to be the result of a past nearby supernova event. A candidate for the reverse shock wave is the supernova remnant North Polar Spur, with an estimated age of 75,000 years and a distance of 130 ± 75 parsecs (424 light years),42 conveniently located in the north sky from where it would have preferentially irradiated the Northern Hemisphere. Assuming the Taylor flux is average and 1,000 neutrons are produced per erg of gamma-ray energy,43 the catastrophe would have released about 10^16 erg/cm 2 (2 x 10^8 cal/cm 2 ), corresponding to a solar flare of 10^43 ergs or a gamma-flash of 10^54 ergs from a supernova about 1 parsec away.
The geographical distribution of particle tracks, 235 U depletion, and 239 Pu concentration shown in Fig. 3 are quite consistent, although the particle tracks seem to be confined to a smaller geographic area. They indicate energy released over the northeastern sector of the U.S., with maximum energy at about 43° N, 85° W, the Michigan area of the Great Lakes region.
A history of suspected cosmic cataclysms over the ages
Wdowczyk and Wolfendale 44 and Zook 36 propose, based on the existing record of solar flare intensities, that solar flares as large as 3 x 10^38 ergs should be expected every 100,000 years. Clark et al. estimate that supernovas release 10^47 10^50 ergs within 10 parsecs of Earth every 100 million years.45 Brackenridge suggests that a supernova impacted the earth in Paleoindian times.46 Damon et al. report evidence from the 14 C tree ring record that SN1006, which occurred at a distance of 1300 par-secs, produced a neutron shower of 2 x 10^8 n/cm 2 . 47 Castagnoli et al. report evidence of the past six nearby supernovae from the thermoluminescence record of Tyrrhenian sea sediments.48 Dar et al. suggest that a cosmic ray jet within 1000 parsec would produce 10^12 muons/cm 2 (greater than 3 x 10^9 eV) and 10^10 protons and neutrons/cm 2 (greater than 10^6 eV) and deposit over 10^12 erg/cm 2 in the atmosphere every 100 million years.49 A cosmic ray jet is also predicted to produce heavy elements via the r-process and could be a source of 235 U enriched up to 60 percent in uranium.
The Paleoindian catastrophe was large by standards of all suspected cosmic occurrences. Normal geomagnetic conditions would focus cosmic rays towards the magnetic poles, concentrating their severity in those regions. However, low magnetic field intensity during a geomagnetic excursion may have allowed excessive cosmic rays to strike northeastern North America. (Whether the geomagnetic excursion admitted cosmic radiation, or the radiation caused the excursion, is uncertain. Given our present state of knowledge, cause and effect in this instance are unclear.) The presence of a nearby small and dense interstellar cloud may explain the origin of the particle bombardment.50 The size of the initial catastrophe may be too large for a solar flare, but a sufficiently powerful nearby supernova or cosmic ray jet could account for it. It appears that the catastrophe initiated a sequence of events that may have included solar flares, impacts, and secondary cosmic ray bombardments.
A devastating effect on Earth
The enormous energy released by the catastrophe at 12,500 yr B.P. could have heated the atmosphere to over 1000°C over Michigan, and the neutron flux at more northern locations would have melted considerable glacial ice. Radiation effects on plants and animals exposed to the cosmic rays would have been lethal, comparable to being irradiated in a 5-megawatt reactor more than 100 seconds.
The overall pattern of the catastrophe matches the pattern of mass extinction before Holocene times. The Western Hemisphere was more affected than the Eastern, North America more than South America, and eastern North America more than western North America.51,52,53 Extinction in the Great Lakes area was more rapid and pronounced than elsewhere. Larger animals were more affected than smaller ones, a pattern that conforms to the expectation that radiation exposure affects large bodies more than smaller ones.54,55 Sharp fluctuations of 14 C in the Icelandic marine sediments at each geomagnetic excursion are interesting; because global carbon deposits in the ocean sediments at a rate of only about 0.0005 percent a year, a sudden increase in sediment 14 C may reflect the rapid die-off of organisms that incorporated radiocarbon shortly after bombardment.
Massive radiation would be expected to cause major mutations in plant life. Maize probably evolved by macro-mutation at that time,55,56 and plant domestication of possibly mutated forms appears worldwide after the Late Glacial period. For example, there was a rapid transition from wild to domesticated grains in the Near East after the catastrophe.57
Implications for future study
Much of what we assume about the Paleoindian period and the peopling of the Americas has been inferred from conventional radiocarbon chronology, which often conflicts with archaeological evidence. This work mandates that conventional radio-carbon dates be reinterpreted in light of hard terrestrial evidence of exposure of the radiocarbon samples to a cosmological catastrophe that affected vast areas of North America and beyond. A nuclear catastrophe can reset a group of unrelated artifacts to a common younger date, creating gaps and false episodes in the fossil record. Geographical variation and complicated overburdens may further confuse the interpretation. Scrutiny of Paleoindian artifacts and the North American paleolandscape, associated stratigraphic sediments, coupled with continued radiological investigations, may provide more evidence for the cosmic catastrophe and new clues to the origin of Paleoindians.
How to contact the principals in this article:
Richard B. Firestone e-mail: firstname.lastname@example.org
William H. Topping
P.O. Box 62
Baldwin, MI. 49304 USA
This paper results from dissertation research that began in 1990, most recently funded by a National Science Foundation Physics Division, by William Topping. Support of Richard Firestone by the Director, Office of Energy Research, Division of Nuclear Physics, of the Office of High Energy and Nuclear Physics of the U.S. Department of Energy is greatly appreciated. The contributions of particular individuals over the years have been invaluable. Tony Baker, Kurt Carr, Chris Ellis, Mima Kapches, Ronald Lesher, Donald B. Simons, James Taylor, Curtis Tomak, John Tomenchuk, and Henry Wright in particular should be thanked for their contributions of artifacts which provided essential information. Alan Smith contributed important experimental data for this paper. We particularly acknowledge the participation of the Royal Ontario Museum and the Smithsonian Institution. In addition, there have been many invaluable contributions of time, analysis, and commentary by physicists, archaeologists, and geologists from the National Superconducting Cyclotron Laboratory at Michigan State University, Phoenix Memorial Laboratory and the Department of Physics at the University of Michigan, Departments of Anthropology and Geology at Wayne State University, Department of Physics at Washington University in St. Louis, Museum of Anthropology at the University of Michigan, Department of Physics at the University of Arizona, Harvard Cyclotron at Harvard University, Oak Ridge National Laboratory, Los Alamos National Laboratory, Johnson Space Center, the State University of Pennsylvania, Lawrence Livermore National Laboratory, and the Lawrence Berkeley National Laboratory.
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